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Ancient texts and archaeological evidence indicate substantial lead exposure during antiquity that potentially impacted human health. Although lead exposure routes were many and included the use of glazed tablewares, paints, cosmetics, and even intentional ingestion, the most significant for the nonelite, rural majority of the population may have been through background air pollution from mining and smelting of silver and lead ores that underpinned the Roman economy. Here, we determined potential health effects of this air pollution using Arctic ice core measurements of Roman-era lead pollution, atmospheric modeling, and modern epidemiology-based relationships between air concentrations, blood lead levels (BLLs), and cognitive decline. Findings suggest air lead concentrations exceeded 150 ng/m³near metallurgical emission sources, with average enhancements of >1.0 ng/m³over Europe during the Pax Romana apogee of the Roman Empire. The result was blood lead enhancements in young children of about 2.4 µg/dl above an estimated Neolithic background of 1.0 µg/dl, leading to widespread cognitive decline including a 2.5-to-3 point reduction in intelligence quotient throughout the Roman Empire. 

Abstract Estimating fire emissions prior to the satellite era is challenging because observations are limited, leading to large uncertainties in the calculated aerosol climate forcing following the preindustrial era. This challenge further limits the ability of climate models to accurately project future climate change. Here, we reconstruct a gridded dataset of global biomass burning emissions from 1750 to 2010 using inverse analysis that leveraged a global array of 31 ice core records of black carbon deposition fluxes, two different historical emission inventories as a priori estimates, and emission-deposition sensitivities simulated by the atmospheric chemical transport model GEOS-Chem. The reconstructed emissions exhibit greater temporal variabilities which are more consistent with paleoclimate proxies. Our ice core constrained emissions reduced the uncertainties in simulated cloud condensation nuclei and aerosol radiative forcing associated with the discrepancy in preindustrial biomass burning emissions. The derived emissions can also be used in studies of ocean and terrestrial biogeochemistry. 

Abstract Black carbon emitted by incomplete combustion of fossil fuels and biomass has a net warming effect in the atmosphere and reduces the albedo when deposited on ice and snow; accurate knowledge of past emissions is essential to quantify and model associated global climate forcing. Although bottom-up inventories provide historical Black Carbon emission estimates that are widely used in Earth System Models, they are poorly constrained by observations prior to the late 20th century. Here we use an objective inversion technique based on detailed atmospheric transport and deposition modeling to reconstruct 1850 to 2000 emissions from thirteen Northern Hemisphere ice-core records. We find substantial discrepancies between reconstructed Black Carbon emissions and existing bottom-up inventories which do not fully capture the complex spatial-temporal emission patterns. Our findings imply changes to existing historical Black Carbon radiative forcing estimates are necessary, with potential implications for observation-constrained climate sensitivity. 

This data set is part of a joint international effort for the East GReenland Ice-core Project (EGRIP), which has retrieved an ice core by drilling through the Northeast Greenland Ice Stream (NEGIS, 75.63°N (North), 35.98°W (West)). Ice streams are responsible for draining a significant fraction of the ice from the Greenland Ice Sheet (GIS), and the project was developed to gain new and fundamental information on ice stream dynamics, thereby improving the understanding of how ice streams will contribute to future sea-level change. The drilled core also provides a new record of past climatic conditions from the northeastern part of the GIS. The project has many international partners and is managed by the Centre for Ice and Climate, Denmark with air support carried out by US ski-equipped Hercules aircraft managed through the US (United States) Office of Polar Programs, National Science Foundation. As of May 2022, approximately 2099.2 m (meters) of ice core have been recovered from the combined efforts of drilling operations in 2017, 2018, and 2019. Here we present records of stable isotopes of oxygen and hydrogen from 21.5 meters to 2120.7 m depth. Bedrock is estimated to be at a depth of approximately 2550 m; the remaining ice is expected to be recovered in the 2022 and 2023 field seasons. The data product presented here is supported by the National Science Foundation project: Collaborative Research: The fingerprint of abrupt temperature events throughout Greenland during the last glacial period. Award # 1804098. 

This data set is part of a joint international effort for the East GReenland Ice-core Project (EGRIP), which has retrieved an ice core by drilling through the Northeast Greenland Ice Stream (NEGIS, 75.63°N (North), 35.98°W (West)). Ice streams are responsible for draining a significant fraction of the ice from the Greenland Ice Sheet (GIS), and the project was developed to gain new and fundamental information on ice stream dynamics, thereby improving the understanding of how ice streams will contribute to future sea-level change. The drilled core also provides a new record of past climatic conditions from the northeastern part of the GIS. The project has many international partners and is managed by the Centre for Ice and Climate, Denmark with air support carried out by US ski-equipped Hercules aircraft managed through the US (United States) Office of Polar Programs, National Science Foundation. As of May 2022, approximately 2099.2 m (meters) of ice core have been recovered from the combined efforts of drilling operations in 2017, 2018, and 2019. Here we present records of stable isotopes of oxygen and hydrogen from 21.5 meters to 2120.7 m depth. Bedrock is estimated to be at a depth of approximately 2550 m; the remaining ice is expected to be recovered in the 2022 and 2023 field seasons. The data product presented here is supported by the National Science Foundation project: Collaborative Research: The fingerprint of abrupt temperature events throughout Greenland during the last glacial period. Award # 1804098. 

The assassination of Julius Caesar in 44 BCE triggered a power struggle that ultimately ended the Roman Republic and, eventually, the Ptolemaic Kingdom, leading to the rise of the Roman Empire. Climate proxies and written documents indicate that this struggle occurred during a period of unusually inclement weather, famine, and disease in the Mediterranean region; historians have previously speculated that a large volcanic eruption of unknown origin was the most likely cause. Here we show using well-dated volcanic fallout records in six Arctic ice cores that one of the largest volcanic eruptions of the past 2,500 y occurred in early 43 BCE, with distinct geochemistry of tephra deposited during the event identifying the Okmok volcano in Alaska as the source. Climate proxy records show that 43 and 42 BCE were among the coldest years of recent millennia in the Northern Hemisphere at the start of one of the coldest decades. Earth system modeling suggests that radiative forcing from this massive, high-latitude eruption led to pronounced changes in hydroclimate, including seasonal temperatures in specific Mediterranean regions as much as 7 °C below normal during the 2 y period following the eruption and unusually wet conditions. While it is difficult to establish direct causal linkages to thinly documented historical events, the wet and very cold conditions from this massive eruption on the opposite side of Earth probably resulted in crop failures, famine, and disease, exacerbating social unrest and contributing to political realignments throughout the Mediterranean region at this critical juncture of Western civilization. 

Abstract. The last glacial period is characterized by a number of millennial climateevents that have been identified in both Greenland and Antarctic ice coresand that are abrupt in Greenland climate records. The mechanisms governingthis climate variability remain a puzzle that requires a precisesynchronization of ice cores from the two hemispheres to be resolved.Previously, Greenland and Antarctic ice cores have been synchronizedprimarily via their common records of gas concentrations or isotopes fromthe trapped air and via cosmogenic isotopes measured on the ice. In thiswork, we apply ice core volcanic proxies and annual layer counting toidentify large volcanic eruptions that have left a signature in bothGreenland and Antarctica. Generally, no tephra is associated with thoseeruptions in the ice cores, so the source of the eruptions cannot beidentified. Instead, we identify and match sequences of volcanic eruptionswith bipolar distribution of sulfate, i.e. unique patterns of volcanicevents separated by the same number of years at the two poles. Using thisapproach, we pinpoint 82 large bipolar volcanic eruptions throughout thesecond half of the last glacial period (12–60 ka). Thisimproved ice core synchronization is applied to determine the bipolarphasing of abrupt climate change events at decadal-scale precision. Inresponse to Greenland abrupt climatic transitions, we find a response in theAntarctic water isotope signals (δ18O and deuterium excess)that is both more immediate and more abrupt than that found with previousgas-based interpolar synchronizations, providing additional support for ourvolcanic framework. On average, the Antarctic bipolar seesaw climateresponse lags the midpoint of Greenland abrupt δ18O transitionsby 122±24 years. The time difference between Antarctic signals indeuterium excess and δ18O, which likewise informs the timeneeded to propagate the signal as described by the theory of the bipolarseesaw but is less sensitive to synchronization errors, suggests anAntarctic δ18O lag behind Greenland of 152±37 years.These estimates are shorter than the 200 years suggested by earliergas-based synchronizations. As before, we find variations in the timing andduration between the response at different sites and for different eventssuggesting an interaction of oceanic and atmospheric teleconnection patternsas well as internal climate variability.